A soft adhesive layer bonded between two rigid substrates, which are being pulled apart, may exhibit diverse instability phenomena before failure, such as cavitation, fingering, and fringe instability. In this study, by subdividing the soft layers into different numbers of disconnected smaller parts, we achieve desired instability modes and mechanical responses of the layer. The partition process not only retains the monotonicity on the tensile curve but also tunes the modulus and stretchability of the adhesive layer. Meanwhile, cavitation in layers of large aspect ratios is suppressed, and the hysteresis during cyclic loading is reduced. This study provides a guideline for the structural design of soft joints and adhesive layers.

References

1.
Liu
,
X.
,
Tang
,
T.-C.
,
Tham
,
E.
,
Yuk
,
H.
,
Lin
,
S.
,
Lu
,
T. K.
, and
Zhao
,
X.
,
2017
, “
Stretchable Living Materials and Devices With Hydrogel–Elastomer Hybrids Hosting Programmed Cells
,”
Proc. Natl. Acad. Sci. U.S.A.
,
114
(
9
), pp.
2200
2205
.
2.
Ahmed
,
G.
, and
Ahmed
,
E.
,
2018
, “
On the Role of the Plaque Porous Structure in Mussel Adhesion: Implications for Adhesion Control Using Bulk Patterning
,”
J. Appl. Mech.
,
85
(
12
),
121003
.
3.
Creton
,
C.
, and
Ciccotti
,
M.
,
2016
, “
Fracture and Adhesion of Soft Materials: A Review
,”
Rep. Prog. Phys.
,
79
(
4
),
046601
.
4.
Shull
,
K. R.
,
2002
, “
Contact Mechanics and the Adhesion of Soft Solids
,”
Mater. Sci. Eng. R
,
36
(
1
), pp.
1
45
.
5.
Yuk
,
H.
,
Lin
,
S.
,
Ma
,
C.
,
Takaffoli
,
M.
,
Fang
,
N. X.
, and
Zhao
,
X.
,
2017
, “
Hydraulic Hydrogel Actuators and Robots Optically and Sonically Camouflaged in Water
,”
Nat. Commun.
,
8
,
14230
.
6.
Ball
,
J. M.
,
1982
, “
Discontinuous Equilibrium Solutions and Cavitation in Nonlinear Elasticity
,”
Philos. Trans. R. Soc. B
,
306
, pp.
557
611
.
7.
Lopez-Pamies
,
O.
,
Idiart
,
M. I.
, and
Nakamura
,
T.
,
2011
, “
Cavitation in Elastomeric Solids: I—A Defect-Growth Theory
,”
J. Mech. Phys. Solids
,
59
(
8
), pp.
1464
1487
.
8.
Zimberlin
,
J. A.
, and
Crosby
,
A. J.
,
2010
, “
Water Cavitation of Hydrogels
,”
J. Polym. Sci. Part B Polym. Phys.
,
48
(
13
), pp.
1423
1427
.
9.
Zimberlin
,
J. A.
,
Sanabriadelong
,
N.
,
Tew
,
G. N.
, and
Crosby
,
A. J.
,
2007
, “
Cavitation Rheology for Soft Materials
,”
Soft Matter
,
3
(
6
), pp.
763
767
.
10.
Long
,
R.
, and
Hui
,
C. Y.
,
2010
, “
Effects of Triaxiality on the Growth of Crack-Like Cavities in Soft Incompressible Elastic Solids
,”
Soft Matter
,
6
(
6
), pp.
1238
1245
.
11.
Overvelde
,
J. T. B.
,
Dykstra
,
D. M. J.
,
de Rooij
,
R.
,
Weaver
,
J.
, and
Bertoldi
,
K.
,
2016
, “
Tensile Instability in a Thick Elastic Body
,”
Phys. Rev. Lett.
,
117
(
9
),
094301
.
12.
Lin
,
S.
,
Mao
,
Y.
,
Radovitzky
,
R.
, and
Zhao
,
X.
,
2017
, “
Instabilities in Confined Elastic Layers Under Tension: Fringe, Fingering and Cavitation
,”
J. Mech. Phys. Solids
,
106
, pp.
229
256
.
13.
Crosby
,
A. J.
,
Shull
,
K. R.
,
Lakrout
,
H.
, and
Creton
,
C.
,
2000
, “
Deformation and Failure Modes of Adhesively Bonded Elastic Layers
,”
J. Appl. Phys.
,
88
(
5
), pp.
2956
2966
.
14.
Lin
,
S.
,
Cohen
,
T.
,
Zhang
,
T.
,
Yuk
,
H.
,
Abeyaratne
,
R.
, and
Zhao
,
X.
,
2016
, “
Fringe Instability in Constrained Soft Elastic Layers
,”
Soft Matter
,
12
(
43
), pp.
8899
8906
.
15.
Chung
,
J. Y.
, and
Chaudhury
,
M. K.
,
2005
, “
Soft and Hard Adhesion
,”
J. Adhes.
,
81
(
10–11
), pp.
1119
1145
.
16.
Chakrabarti
,
A.
, and
Chaudhury
,
M. K.
,
2013
, “
Direct Measurement of the Surface Tension of a Soft Elastic Hydrogel: Exploration of Elastocapillary Instability in Adhesion
,”
Langmuir
,
29
(
23
), pp.
6926
6935
.
17.
Chaudhury
,
M. K.
,
Chakrabarti
,
A.
, and
Ghatak
,
A.
,
2015
, “
Adhesion-Induced Instabilities and Pattern Formation in Thin Films of Elastomers and Gels
,”
Eur. Phys. J. E
,
38
(
7
), pp.
1
26
.
18.
Animangsu
,
A. G.
, and
Chaudhury
,
M. K.
,
2003
, “
Adhesion-Induced Instability Patterns in Thin Confined Elastic Film
,”
Langmuir
,
19
(
7
), pp.
2621
2631
.
19.
Webber
,
R. E.
,
Shull
,
K. R.
,
Roos
,
A.
, and
Creton
,
C.
,
2003
, “
Effects of Geometric Confinement on the Adhesive Debonding of Soft Elastic Solids
,”
Phys. Rev. E
,
68
(
1
),
021805
.
20.
Shull
,
K. R.
, and
Creton
,
C.
,
2004
, “
Deformation Behavior of Thin, Compliant Layers Under Tensile Loading Conditions
,”
J. Polym. Sci. Part B: Polym. Phys.
,
42
(
22
), pp.
4023
4043
.
21.
Dollhofer
,
J.
,
Chiche
,
A.
,
Muralidharan
,
V.
,
Creton
,
C.
, and
Hui
,
C. Y.
,
2004
, “
Surface Energy Effects for Cavity Growth and Nucleation in an Incompressible Neo-Hookean Material––Modeling and Experiment
,”
Int. J. Solids Struct.
,
41
(
22–23
), pp.
6111
6127
.
22.
Gent
,
A. N.
, and
Lindley
,
P. B.
,
1959
, “
Internal Rupture of Bonded Rubber Cylinders in Tension
,”
Proc. R. Soc. Lond.
,
249
(
1257
), pp.
195
205
.
23.
Chiche
,
A.
,
Dollhofer
,
J.
, and
Creton
,
C.
,
2005
, “
Cavity Growth in Soft Adhesives
,”
Eur. Phys. J. E
,
17
(
4
), pp.
389
401
.
24.
Biwa
,
S.
,
2006
, “
Cavitation in Finite Elasticity With Surface Energy Effects
,”
Int. J. Non-Linear Mech.
,
41
(
9
), pp.
1084
1094
.
25.
Fond
,
C.
,
2001
, “
Cavitation Criterion for Rubber Materials: A Review of Void-Growth Models
,”
J. Polym. Sci. Part B Polym. Phys.
,
39
(
17
), pp.
2081
2096
.
26.
Pourmodheji
,
R.
,
Qu
,
S.
, and
Yu
,
H.
,
2018
, “
Two Possible Defect Growth Modes in Soft Solids
,”
J. Appl. Mech.
,
85
(
3
),
031001
.
27.
Shull
,
K. R.
,
Flanigan
,
C. M.
, and
Crosby
,
A. J.
,
2000
, “
Fingering Instabilities of Confined Elastic Layers in Tension
,”
Phys. Rev. Lett.
,
84
(
14
), pp.
3057
3060
.
28.
Biggins
,
J. S.
,
Saintyves
,
B.
,
Wei
,
Z.
,
Bouchaud
,
E.
, and
Mahadevan
,
L.
,
2013
, “
Digital Instability of a Confined Elastic Meniscus
,”
Proc. Natl. Acad. Sci. U.S.A.
,
110
(
31
), pp.
12545
12548
.
29.
Saintyves
,
B.
,
Dauchot
,
O.
, and
Bouchaud
,
E.
,
2013
, “
Bulk Elastic Fingering Instability in Hele-Shaw Cells
,”
Phys. Rev. Lett.
,
111
(
4
), pp.
2466
2472
.
30.
Mao
,
G.
,
Wu
,
L.
,
Liang
,
X.
, and
Qu
,
S.
,
2017
, “
Morphology of Voltage-Triggered Ordered Wrinkles of a Dielectric Elastomer Sheet
,”
J. Appl. Mech.
,
84
(
11
),
111005
.
31.
Diani
,
J.
,
Fayolle
,
B.
, and
Gilormini
,
P.
,
2009
, “
A Review on the Mullins Effect
,”
Eur. Polym. J.
,
45
(
3
), pp.
601
612
.
32.
Cristiano
,
A.
,
Marcellan
,
A.
,
Long
,
R.
,
Hui
,
C. Y.
,
Stolk
,
J.
, and
Creton
,
C.
,
2010
, “
An Experimental Investigation of Fracture by Cavitation of Model Elastomeric Networks
,”
J. Polym. Sci. Part B Polym. Phys.
,
48
(
13
), pp.
1409
1422
.
33.
Li
,
J.
,
Celiz
,
A. D.
,
Yang
,
J.
,
Yang
,
Q.
,
Wamala
,
I.
,
Whyte
,
W.
,
Seo
,
B. R.
,
Vasilyev
,
N. V.
,
Vlassak
,
J. J.
, and
Suo
,
Z.
,
2017
, “
Tough Adhesives for Diverse Wet Surfaces
,”
Science
,
357
(
6349
), pp.
378
381
.
34.
Lin
,
S.
,
Mao
,
Y.
,
Yuk
,
H.
, and
Zhao
,
X.
,
2018
, “
Material-Stiffening Suppresses Elastic Fingering and Fringe Instabilities
,”
Int. J. Solids Struct.
,
139–140
, pp.
96
104
.
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